江林教授、彭美文副教授及其合作者在Adv. Funct. Mater.上发表论文

发布时间:2025-12-25访问量:10设置


题目:

Decoupling Mass Transport Conflicts in Solar Driven Water-Salt Co-Production via Heterogeneous Evaporation Interface

作者:

He Yang1#, Xuan Wang1#, Shihua Li1, Bo Zhao4, Chang Liu1, Dong Li1, Zhiqiang Liang1, Ibrahim Abdulhalim5, Meiwen Peng1*, Yinghui Sun2,3* & Lin Jiang1*

单位:

1State Key Laboratory of Bioinspired Interfacial Materials Science, Institute of Functional Nano and Soft Materials (FUNSOM), Soochow University, Suzhou, 215123, China.

2Innovation Centre for Chemical Sciences, College of Chemistry, Chemical Engineering and Materials Science, Soochow University, Suzhou, 215123, China.

3Key Laboratory of Science and Engineering for the Multi-modal, Prevention and Control of Major Chronic Diseases

Ministry of Industry and Information Technology, Zhengzhou, 450000, China.

4Macao Institute of Materials Science and Engineering (MIMSE), Faculty of Innovation Engineering, Macau University of Science and Technology, Macau, 999078, China.

5Department of Electrooptics and Photonics Engineering and the Ilse-Katz, Center for Nanoscale Science and Technology, ECE School, Ben Gurion University, Beer Sheva, 84105, Israel.

摘要:

Efficient water-salt co-production is crucial for treating high-concentration brine, yet remains challenging due to conflicting mass transport demands. High evaporation rate requires enhanced mass transfer to achieve salt tolerance, whereas high salt production rate demands restricted transport for salt nucleation. Due to the inherent mass transport conflict, current reported homogeneous evaporation interfaces with single mass transfer properties create a wide water-salt interference area, resulting in inevitably low water-salt co-production performance. Herein, this study develops a solar evaporator with a heterogeneous evaporation interface (HE-EI) that achieves an impressive evaporation rate of 3.36 kg·m−2·h−1 and salt production rate of 0.52 kg·m−2·h−1 for high-concentrated brine (20 wt.% NaCl) under 1 kW·m−2 illumination, outperforming reported water-salt co-production evaporators. Experimental results and theoretical analyses demonstrate that the HE-EI has a very narrow water-salt interference area, effectively decoupling mass transport conflicts and thereby achieving superior water-salt co-production performance. Notably, when the solar evaporator with HE-EI is used for lithium extraction from salt-lake brine, the enrichment rate of Li+ is 240 times higher than simulated evaporation ponds, enabling Li salt crystallization within the salt-producing area. Overall, this HE-EI addresses the long-standing conflicts between water-salt co-production, opening a scalable pathway toward the global challenge of high-concentration brine treatment.

影响因子:

19.0

分区情况:

一区

链接:

https://doi.org/10.1002/adfm.202520083



责任编辑:郭佳


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